Rep. Math. Phys. 43, 283 (1999)
A. Orłowski
The usefulness of Wehrl's entropy in quantum optics is investigated. Possible applications to the classification of quantum states with respect to their statistical properties are presented. A general variational proof of the observation that for a given average photon number the maximum Wehrl's entropy is attained for thermal states is given.
May 29, 1998
Mar 18, 1998
Changes of the electrokinetic effects induced by guided light in capillary electrophoresis
Electrophoresis 20, 2493-2500 (1999)
Leonardo De Boni, Lilian T. C. França, Hans-Peter H. Grieneisen, Maciej Janowicz, Tarso B. L. Kist, Angelica R. Consiglio, Júlio R. Schoffen, Valter Stefani, Carlos Termignoni
The phenomenon of electrophoresis in free solution has been studied theoretically down to the molecular level for decades. In addition, intermolecular photo-induced proton transfer reactions, which occur in a wide class of molecules (phenols and aminoarenes) as well as proteins (green fluorescent protein), were also studied extensively. However, the study of the effect of light-induced electrophoretic mobility changes of the analytes in electrophoresis was begun only recently. In the present work, capillary zone electrophoresis was chosen as the environment to measure the magnitude of these electrophoretic mobility shifts induced by light. Background electrolytes (running electrolytes) with high refractive indices were developed, allowing the capillary to work like an optical fiber. The experimental conditions for obtaining stable coupling and guided laser light along the liquid core are discussed. Experimental evidence of band compression is observed, leading to a solitary wave behavior of the analyte band (2-naphthol). These solitary waves result from competition between thermal diffusion (dispersion mechanism) and a nonlinear (band compression) effect due to the combined electrophoresis phenomenon and absorption of guided light by the molecules of the band (which are subjected to a reversible intermolecular proton transfer reaction as one of their decay routes). The possibilities of applying this effect to different methods and techniques are also discussed.
Leonardo De Boni, Lilian T. C. França, Hans-Peter H. Grieneisen, Maciej Janowicz, Tarso B. L. Kist, Angelica R. Consiglio, Júlio R. Schoffen, Valter Stefani, Carlos Termignoni
The phenomenon of electrophoresis in free solution has been studied theoretically down to the molecular level for decades. In addition, intermolecular photo-induced proton transfer reactions, which occur in a wide class of molecules (phenols and aminoarenes) as well as proteins (green fluorescent protein), were also studied extensively. However, the study of the effect of light-induced electrophoretic mobility changes of the analytes in electrophoresis was begun only recently. In the present work, capillary zone electrophoresis was chosen as the environment to measure the magnitude of these electrophoretic mobility shifts induced by light. Background electrolytes (running electrolytes) with high refractive indices were developed, allowing the capillary to work like an optical fiber. The experimental conditions for obtaining stable coupling and guided laser light along the liquid core are discussed. Experimental evidence of band compression is observed, leading to a solitary wave behavior of the analyte band (2-naphthol). These solitary waves result from competition between thermal diffusion (dispersion mechanism) and a nonlinear (band compression) effect due to the combined electrophoresis phenomenon and absorption of guided light by the molecules of the band (which are subjected to a reversible intermolecular proton transfer reaction as one of their decay routes). The possibilities of applying this effect to different methods and techniques are also discussed.
Dec 19, 1997
Suppression of the Rabi oscillations in a cavity partially filled with a dielectric having a time-dependent refractive index
In this paper the dynamics of wave fields in a cavity, part of which is filled with a dielectric, are investigated. The wave equation is solved approximately using the method of multiple time scales. Phase modulations of the cavity modes in an adiabatic case are given up to the first order. A simple effective field Hamiltonian operator is derived and then used to analyze the interaction of radiation with a two-level atom passing through the cavity. Corrections to the Rabi oscillations due to the time-dependent frequency of the cavity photons are investigated. It is shown that adiabatic time dependence of the refractive index of the dielectric can lead to suppression of the Rabi oscillations of atomic inversion.
Physical Review A 57, 5016 (1998)
Physical Review A 57, 5016 (1998)
Jun 16, 1997
Radiative decay of Trojan wave packets
Zofia Bialynicka-Birula and Iwo Bialynicki-Birula
We calculate the decay rates due to spontaneous emission for electronic states described by Trojan wave packets. The spontaneous decay rate for a typical Trojan state (n=60) is six orders of magnitude smaller than the ionization rate and it is about one order of magnitude smaller than the rate for the corresponding ordinary circular Rydberg state.
Phys. Rev. A 56, 3623 (1997)
We calculate the decay rates due to spontaneous emission for electronic states described by Trojan wave packets. The spontaneous decay rate for a typical Trojan state (n=60) is six orders of magnitude smaller than the ionization rate and it is about one order of magnitude smaller than the rate for the corresponding ordinary circular Rydberg state.
Phys. Rev. A 56, 3623 (1997)
Feb 6, 1997
Band of localized electromagnetic waves in random arrays of dielectric cylinders
Marian Rusek, Arkadiusz Orłowski, and Jan Mostowski
Anderson localization of electromagnetic waves in random arrays of dielectric cylinders is studied. An effective theoretical approach based on analysis of probability distributions, not averages, is developed. The disordered dielectric medium is modeled by a system of randomly distributed two-dimensional electric dipoles. Spectra of certain random matrices are investigated and the appearance of the band of localized waves emerging in the limit of an infinite medium is discovered. It suggests deeper insight into the existing experimental results.
Phys. Rev. E 56, 4892 (1997)
Anderson localization of electromagnetic waves in random arrays of dielectric cylinders is studied. An effective theoretical approach based on analysis of probability distributions, not averages, is developed. The disordered dielectric medium is modeled by a system of randomly distributed two-dimensional electric dipoles. Spectra of certain random matrices are investigated and the appearance of the band of localized waves emerging in the limit of an infinite medium is discovered. It suggests deeper insight into the existing experimental results.
Phys. Rev. E 56, 4892 (1997)
Nov 5, 1996
Rotational frequency shift
Iwo Bialynicki-Birula and Zofia Bialynicka-Birula
The notion of the rotational frequency shift, an analog of the Doppler shift, is introduced. This new frequency shift occurs for atomic systems that lack rotational invariance, but have stationary states in a rotating frame. The rotational frequency shift is given by the scalar product of the angular velocity and the angular momentum of the emitted photon in full analogy with the standard Doppler shift which is given by the scalar product of the linear velocity of the source and the linear momentum of the photon. The rotational frequency shift can be observed only in a Mössbauer-like regime when the angular recoil is negligible.
Phys. Rev. Lett. 78, 2539 (1997)
The notion of the rotational frequency shift, an analog of the Doppler shift, is introduced. This new frequency shift occurs for atomic systems that lack rotational invariance, but have stationary states in a rotating frame. The rotational frequency shift is given by the scalar product of the angular velocity and the angular momentum of the emitted photon in full analogy with the standard Doppler shift which is given by the scalar product of the linear velocity of the source and the linear momentum of the photon. The rotational frequency shift can be observed only in a Mössbauer-like regime when the angular recoil is negligible.
Phys. Rev. Lett. 78, 2539 (1997)
May 30, 1996
Numerical studies of the dynamics of multiphoton processes with arbitrary field polarization: Methodological considerations
Etienne Huens, Bernard Piraux, Alejandro Bugacov, Mariusz Gajda
We describe an approach of spectral type for numerically integrating the time-dependent Schrödinger equation associated to the interaction of a one active electron atom with an electromagnetic pulsed field whose polarization may be arbitrary. The wave function is represented on a Coulomb-Sturmian basis. The time propagation method is based on a parallel-iterated Runge-Kutta method of predictor-corrector type. This method is in fact fully implicit and of very high order, ensuring a high stability of the time propagation. Moreover, it has the following advantages: it provides a scheme for an adaptive time step and it is particularly well suited to parallel computing. We discuss the performance of the present approach and compare it to already existing ones. In the case of linearly polarized fields, most of our results are in good agreement with those obtained with other approaches. In the case of circularly polarized fields, we compare our results with those obtained by, so far, the only existing method which is based on the single state Floquet approximation. Finally, and for the sake of illustration, we treat the case of the interaction of atomic hydrogen with a strong pulsed electromagnetic field whose polarization depends on time.
Phys. Rev. A 55, 2132 (1997)
We describe an approach of spectral type for numerically integrating the time-dependent Schrödinger equation associated to the interaction of a one active electron atom with an electromagnetic pulsed field whose polarization may be arbitrary. The wave function is represented on a Coulomb-Sturmian basis. The time propagation method is based on a parallel-iterated Runge-Kutta method of predictor-corrector type. This method is in fact fully implicit and of very high order, ensuring a high stability of the time propagation. Moreover, it has the following advantages: it provides a scheme for an adaptive time step and it is particularly well suited to parallel computing. We discuss the performance of the present approach and compare it to already existing ones. In the case of linearly polarized fields, most of our results are in good agreement with those obtained with other approaches. In the case of circularly polarized fields, we compare our results with those obtained by, so far, the only existing method which is based on the single state Floquet approximation. Finally, and for the sake of illustration, we treat the case of the interaction of atomic hydrogen with a strong pulsed electromagnetic field whose polarization depends on time.
Phys. Rev. A 55, 2132 (1997)
Jan 1, 1996
Photon generation by time-dependent dielectric: A soluble model
Markus Cirone, Kazimierz Rzążewski and Jan Mostowski
A soluble model of electromagnetic field interacting with time-dependent dielectric medium is given. The main assumption is that the dielectric constant is switched rapidly from the initial to the final value. Generation of electromagnetic field and photon statistics are found.
Phys. Rev. A 55, 62 (1997)
A soluble model of electromagnetic field interacting with time-dependent dielectric medium is given. The main assumption is that the dielectric constant is switched rapidly from the initial to the final value. Generation of electromagnetic field and photon statistics are found.
Phys. Rev. A 55, 62 (1997)
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